Search results for " ADIABATIC PASSAGE"
showing 10 items of 26 documents
Laser control in open molecular systems: STIRAP and Optimal Control
2007
We examine the effect of dissipation on the laser control of a process that transforms a state into a superposed state. We consider a two-dimensional double well of a single potential energy surface. In the context of reactivity, the objective of the control is the localization in a given well, for instance the creation of an enantiomeric form whereas for quantum gates, this control corresponds to one of the transformation of the Hadamard gate. The environment is either modelled by coupling few harmonic oscillators (up to five) to the system or by an effective interaction with an Ohmic bath. In the discrete case, dynamics is carried out exactly by using the coupled harmonic adiabatic channe…
Computational investigation and experimental considerations for the classical implementation of a full adder on SO2 by optical pump-probe schemes
2008
International audience; Following the scheme recently proposed by Remacle and Levine Phys. Rev. A 73, 033820 2006 , we investigate the concrete implementation of a classical full adder on two electronic states X˜ 1A1 and C ˜ 1B2 of the SO2 molecule by optical pump-probe laser pulses using intuitive and counterintuitive stimulated Raman adiabatic passage excitation schemes. The resources needed for providing the inputs and reading out are discussed, as well as the conditions for achieving robustness in both the intuitive and counterintuitive pump-dump sequences. The fidelity of the scheme is analyzed with respect to experimental noise and two kinds of perturbations: The coupling to the neigh…
Connection between optimal control theory and adiabatic-passage techniques in quantum systems
2012
This work explores the relationship between optimal control theory and adiabatic passage techniques in quantum systems. The study is based on a geometric analysis of the Hamiltonian dynamics constructed from the Pontryagin Maximum Principle. In a three-level quantum system, we show that the Stimulated Raman Adiabatic Passage technique can be associated to a peculiar Hamiltonian singularity. One deduces that the adiabatic pulse is solution of the optimal control problem only for a specific cost functional. This analysis is extended to the case of a four-level quantum system.
Contrôle quantique adiabatique : technique de passage adiabatique parallèle et systèmes dissipatifs
2011
The first part of this thesis is devoted to the theoretical analysis of adiabatic processes allowing the transfer of population from an initial state to a target state of a quantum system. The strategy of parallel adiabatic passage, in which the coupling parameters are specifically designed to optimize the adiabatic passage corresponding to parallel eigenvalues at all times, allows one to combine the energetically efficiency of pi-pulse and related strategies with the robustness of standard adiabaticpassage. The second part of this thesis concerns the effects of the dissipation in adiabatic passage. The non-adiabatic transition probability formula of a two state system with dissipation is e…
Two-laser multiphoton adiabatic passage in the frame of the Floquet theory. Applications to (1+1) and (2+1) STIRAP
1998
We develop an adiabatic two-mode Floquet theory to analyse multiphoton coherent population transfer in N-level systems by two delayed laser pulses, which is a generalization of the three-state stimulated Raman adiabatic passage (STIRAP). The main point is that, under conditions of non-crossing and adiabaticity, the outcome and feasibility of a STIRAP process can be determined by the analysis of two features: (i) the lifting of degeneracy of dressed states at the beginning and at the end of the laser pulses, and (ii) the connectivity of these degeneracy-lifted branches in the quasienergy diagram. Both features can be determined by stationnary perturbation theory in the Floquet representation…
Roadmap on STIRAP applications
2019
STIRAP (stimulated Raman adiabatic passage) is a powerful laser-based method, usually involving two photons, for efficient and selective transfer of populations between quantum states. A particularly interesting feature is the fact that the coupling between the initial and the final quantum states is via an intermediate state, even though the lifetime of the latter can be much shorter than the interaction time with the laser radiation. Nevertheless, spontaneous emission from the intermediate state is prevented by quantum interference. Maintaining the coherence between the initial and final state throughout the transfer process is crucial. STIRAP was initially developed with applications in …
Rovibrational controlled-NOT gates using optimized stimulated Raman adiabatic passage techniques and optimal control theory
2009
Implementation of quantum controlled-NOT (CNOT) gates in realistic molecular systems is studied using stimulated Raman adiabatic passage (STIRAP) techniques optimized in the time domain by genetic algorithms or coupled with optimal control theory. In the first case, with an adiabatic solution (a series of STIRAP processes) as starting point, we optimize in the time domain different parameters of the pulses to obtain a high fidelity in two realistic cases under consideration. A two-qubit CNOT gate constructed from different assignments in rovibrational states is considered in diatomic (NaCs) or polyatomic $({\text{SCCl}}_{2})$ molecules. The difficulty of encoding logical states in pure rota…
Zeno-like phenomena in STIRAP processes
2011
The presence of a continuous measurement quantum Zeno effect in a stimulated Raman adiabatic passage is studied, exploring in detail a sort of self-competition of the damping, which drives the system toward a loss of population and, at the same time, realizes the conditions for optimizing the adiabatic passage.
Arbitrary qudit gates by adiabatic passage
2013
We derive an adiabatic technique that implements the most general SU($d$) transformation in a quantum system of $d$ degenerate states, featuring a qudit. This technique is based on the factorization of the SU($d$) transformation into $d$ generalized quantum Householder reflections, each of which is implemented by a two-shot stimulated Raman adiabatic passage with appropriate static phases. The energy of the lasers needed to synthesize a single Householder reflection is shown to be remarkably constant as a function of $d$. This technique is directly applicable to a linear trapped ion system with $d+1$ ions. We implement the quantum Fourier transform numerically in a qudit with $d=4$ (defined…
Generation of entanglement in systems of intercoupled qubits
2014
We consider systems of two and three qubits, mutually coupled by Heisenberg-type exchange interaction and interacting with external laser fields. We show that these systems allow one to create maximally entangled Bell states, as well as three qubit Greenberger-Horne-Zeilinger and W states. In particular, we point out that some of the target states are the eigenstates of the initial bare system. Due to this, one can create entangled states by means of pulse area and adiabatic techniques, when starting from a separable (non-entangled) ground state. On the other hand, for target states, not present initially in the eigensystem of the model, we apply the robust stimulated Raman adiabatic passag…